[en] Radionuclide behavior during various severe accident conditions has been addressed as one of the important issues to discuss environmental safety in nuclear power plants. The present paper deals with the development of analytical models and their validations for the agglomeration of multiple-component aerosol and spray removal that controls source terms to the environment of both aerosols and gaseous radionuclides during recirculation mode operation in a containment system for a light water reactor. As for aerosol agglomeration, the single collision kernel model that can cover all types of two-body collision of aerosol was developed. In addition, the dynamic model that can treat aerosol and vapor transfer leading to the equilibrium condition under the containment spray operation was developed. The validations of the present models for multiple-component aerosol growth by agglomeration were performed by comparisons with Nuclear Safety Pilot Plant (NSPP) experiments at Oak Ridge National Laboratory (ORNL) and AB experiments at Hanford Engineering National Laboratory (HEDL). In addition, the spray removal models were applied to the analysis of containment spray experiment (CSE) at HEDL. The results calculated by the models showed good agreements with experimental results. (author)