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AbstractAbstract
[en] 57Fe Moessbauer spectroscopy was applied to an iron-based layered superconductor LaFeAsO0.89F0.11 with a transition temperature of 26 K and to its parent material LaFeAsO. Throughout the temperature range from 4.2 to 298 K, a singlet pattern with no magnetic splitting was observed in the Moessbauer spectrum of the F-doped superconductor. Furthermore, no additional internal magnetic field was observed for the spectrum measured at 4.2 K under a magnetic field of 7 T. On the other hand, magnetically split spectra were observed in the parent LaFeAsO below 140 K, and this temperature is slightly lower than that of a structural phase transition from tetragonal to orthorhombic phase, which accompanies the electrical resistivity anomaly at around 150 K. The magnetic moment is estimated to be ∼0.35 μB/Fe from the internal magnetic field of 5.3 T at 4.2 K in the orthorhombic phase, and the spin disorder appears to remain in the magnetically ordered state even at 4.2 K. The lack of a magnetic transition in LaFeAsO0.89F0.11 down to 4.2 K suggests that this system exhibits a paramagnetic state or that the magnetic moment is small. The present results show that F doping effectively suppresses the magnetic and structural transitions in the parent material, leading to the emergence of superconductivity in the F-doped system. (author)
Source
Available from doi: http://dx.doi.org/10.1143/JPSJ.77.103706; 16 refs., 4 figs., 1 tab.
Record Type
Journal Article
Journal
Journal of the Physical Society of Japan; ISSN 0031-9015;
; v. 77(10); p. 103706.1-103706.3

Country of publication
ARSENIC COMPOUNDS, CRYSTAL STRUCTURE, CRYSTAL-PHASE TRANSFORMATIONS, FLUORIDES, FLUORINE ADDITIONS, IRON 57, IRON COMPOUNDS, ISOMER SHIFT, LANTHANUM COMPOUNDS, MAGNETIC FIELDS, MAGNETIC MOMENTS, MOESSBAUER EFFECT, ORDER-DISORDER MODEL, OXIDES, OXYGEN COMPOUNDS, PARAMAGNETISM, PNICTIDES, SPIN, SUPERCONDUCTIVITY, SUPERCONDUCTORS, TEMPERATURE DEPENDENCE, TRANSITION TEMPERATURE, X-RAY DIFFRACTION
ANGULAR MOMENTUM, CHALCOGENIDES, COHERENT SCATTERING, DIFFRACTION, ELECTRIC CONDUCTIVITY, ELECTRICAL PROPERTIES, EVEN-ODD NUCLEI, FLUORINE COMPOUNDS, HALIDES, HALOGEN COMPOUNDS, INTERMEDIATE MASS NUCLEI, IRON ISOTOPES, ISOTOPES, MAGNETISM, MATHEMATICAL MODELS, NUCLEAR MODELS, NUCLEI, OXYGEN COMPOUNDS, PARTICLE PROPERTIES, PHASE TRANSFORMATIONS, PHYSICAL PROPERTIES, RARE EARTH COMPOUNDS, SCATTERING, STABLE ISOTOPES, THERMODYNAMIC PROPERTIES, TRANSITION ELEMENT COMPOUNDS
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