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AbstractAbstract
[en] A compact correlation-function expansion is developed for n-order optical susceptibilities in the frequency domain using the Keldysh-Schwinger loop. By not keeping track of the relative time ordering of bra and ket interactions at the two branches of the loop, the resulting expressions contain only n+1 basic terms, compared to the 2n terms required for a fully-time-ordered density matrix description. Superoperator Green's function expressions for χ(n) derived using both expansions reflect different types of interferences between pathways. These are demonstrated for correlation-induced resonances in four-wave-mixing signals
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(c) 2008 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA)
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Journal Article
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