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AbstractAbstract
[en] This work is a contribution to the development of fuel plates for Research Nuclear Reaction Materials Test Reactors. The plates have the core constituted by dispersions of metallic uranium in aluminum. The main topics of this work are: 1) The preparation of uranium powder with particle sizes in the 53-105μm diameter range; 2) The mixture and cold-pressing of uranium and aluminum powders for different uranium concentrations; 3) The behavior of the dispersions in the roll milling conditions; 4) Blister, radiographic, metallographic and irradiation tests for quality control of the plates. The irradiation test was performed in the IEA-R1 swimming-pool reactor using a prototype with a dispersion of aluminum and natural uranium (45 w/o ), reaching an integrated neutron flux of 8.663 X 1018 n/cm2 , no visual changes being noticed after the completion of the experiment. The behavior of the uranium-aluminum reaction for dispersions with 45% w/o uranium also studied. X-ray diffraction experiments showed the formation of UAl2 UAl3 and UAl4, while energy dispersive analysis of X-rays(EDAX) demonstrated that the diffusion of aluminum in uranium is the mechanism responsible for that reaction. The activation energy for the U-Al reaction was determined by dilatometric experiments yielding 20.2 kcal/mol.The aluminum-uranium reaction reaches an end when extended to 96 h at 600 deg C, namely, when all the uranium is found in the UAl4 composition. (author)
Original Title
Desenvolvimento de combustivel tipo placa, com nucleo constituido por dispersao U-Al para reatores de ensaios de materiais
Primary Subject
Source
1979; 101 p; 51 refs., 41 figs., 14 tabs.; Diss. (M.Sc.)
Record Type
Miscellaneous
Literature Type
Thesis/Dissertation
Report Number
Country of publication
ACTINIDES, COHERENT SCATTERING, DIFFRACTION, ELECTROMAGNETIC RADIATION, ELEMENTS, ENERGY SOURCES, ENRICHED URANIUM REACTORS, FUEL ELEMENTS, FUELS, IONIZING RADIATIONS, MATERIALS, METALLURGY, METALS, POOL TYPE REACTORS, RADIATIONS, RADIOACTIVITY, REACTOR COMPONENTS, REACTOR MATERIALS, REACTORS, RESEARCH AND TEST REACTORS, RESEARCH REACTORS, SCATTERING, THERMAL REACTORS, WATER COOLED REACTORS, WATER MODERATED REACTORS
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