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AbstractAbstract
[en] The work presented in this dissertation contains the first observation of spin-resolved resonance fluorescence from a single quantum dot and its application of direct measurement of electron spin dynamics. The Mollow triplet and the Mollow quintuplet, which are the hallmarks of resonance fluorescence, are presented as the non-spin-resolved and spin-resolved resonance fluorescence spectrum, respectively. The negligible laser background contribution, the near pure radiative broadened spectrum and the anti-bunching photon statistics imply the sideband photons are background-free and near transform-limited single photons. This demonstration is a promising step towards the heralded single photon generation and electron spin readout. Instead of resolving spectrum, an alternative spin-readout scheme by counting resonance fluorescence photons under moderate laser power is demonstrated. The measurements of n-shot time-resolved resonance fluorescence readout are carried out to reveal electron spin dynamics of the measurement induced back action and the spin relaxation. Hyperfine interaction and heavy-light hole mixing are identified as the relevant mechanisms for the back action and phonon-assistant spin-orbit interaction dominates the spin relaxation. After a detailed discussion on charge-spin configurations in coupled quantum dots system, the single-shot readout on electron spin are proposed. (orig.)
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18 Nov 2009; 124 p; Diss. (Dr.rer.nat.)
Record Type
Miscellaneous
Literature Type
Thesis/Dissertation
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DE-EXCITATION, ELECTRONS, EMISSION SPECTRA, EV RANGE 01-10, EXCITED STATES, EXCITONS, GALLIUM ARSENIDES, GROUND STATES, INDIUM ARSENIDES, INFRARED SPECTRA, LASER RADIATION, LINE WIDTHS, L-S COUPLING, NEAR INFRARED RADIATION, PHONONS, PHOTON COLLISIONS, QUANTUM DOTS, RELAXATION, RESONANCE FLUORESCENCE, SEMICONDUCTOR MATERIALS, SPIN ORIENTATION, TEMPERATURE RANGE 0000-0013 K
ARSENIC COMPOUNDS, ARSENIDES, COLLISIONS, COUPLING, ELECTROMAGNETIC RADIATION, ELEMENTARY PARTICLES, EMISSION, ENERGY LEVELS, ENERGY RANGE, ENERGY-LEVEL TRANSITIONS, EV RANGE, FERMIONS, FLUORESCENCE, GALLIUM COMPOUNDS, INDIUM COMPOUNDS, INFRARED RADIATION, INTERMEDIATE COUPLING, LEPTONS, LUMINESCENCE, MATERIALS, NANOSTRUCTURES, ORIENTATION, PHOTON EMISSION, PNICTIDES, QUASI PARTICLES, RADIATIONS, SPECTRA, TEMPERATURE RANGE
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