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AbstractAbstract
[en] Radioactivity quantification of gamma-ray emitter radionuclides in samples measured by HPGe gamma-ray spectrometry relies on the analysis of the photopeaks present in the spectra, especially on the accurate determination of their net areas. Such a task is usually performed with the aid of proprietary software tools. This work presents a methodology, algorithm descriptions and an open source application, called OpenGamma, for the peak search and analysis in order to obtain the relevant peaks parameters and radionuclides activities. The computational implementation is released entirely in open-source license for the main code and with the use of open software packages for interface design and mathematical libraries. The procedure for the peak search is performed on a three step approach. Firstly a preliminary search is done by using the second-difference method, consisting in the generation of a derived spectrum in order to find candidate peaks. In the second step, the experimental peaks widths are assessed and well formed and isolated ones are chosen to obtain a FWHM vs. channel relationship, by application of the Levenberg-Marquardt minimization method for non-linear fitting. Lastly, regions of the spectrum with grouped peaks are marked and a non-linear fit is again applied to each region to obtain baseline and photopeaks terms; from these terms, peaks net areas are then assessed. (author)
Original Title
Desenvolvimento de um codigo computacional aberto de analise quantitativa para determinacao de radionuclideos por espectrometria gama com detectores semicondutores
Primary Subject
Source
2010; 101 p; Tese (Ph.D.)
Record Type
Miscellaneous
Literature Type
Thesis/Dissertation; Numerical Data
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