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AbstractAbstract
[en] The 'Atoms for Peace' mission initiated in the mid-1950s paved the way for the development and deployment of nuclear fission reactors as a source of heat energy for electricity generation in nuclear power reactors and as a source of neutrons in non-power reactors for research, materials irradiation, and testing and production of radioisotopes. The fuels for nuclear reactors are manufactured from natural uranium (∼99.3% 238U + ∼0.7% 235U) and natural thorium (∼100% 232Th) resources. Currently, most power and research reactors use 235U, the only fissile isotope found in nature, as fuel. The fertile isotopes 238U and 232Th are transmuted in the reactor to human-made 239Pu and 233U fissile isotopes, respectively. Likewise, minor actinides (MA) (Np, Am and Cm) and other plutonium isotopes are also formed by a series of neutron capture reactions with 238U and 235U. Long term sustainability of nuclear power will depend to a great extent on the efficient, safe and secure utilization of fissile and fertile materials. Light water reactors (LWRs) account for more than 82% of the operating reactors, followed by pressurized heavy water reactors (PHWRs), which constitute ∼10% of reactors. LWRs will continue to dominate the nuclear power market for several decades, as long as economically viable natural uranium resources are available. Currently, the plutonium obtained from spent nuclear fuel is subjected to mono recycling in LWRs as uranium-plutonium mixed oxide (MOX), containing up to 12% PuO2, in a very limited way. The reprocessed uranium (RepU) is also re-enriched and recycled in LWRs in a few countries. Unfortunately, the utilization of natural uranium resources in thermal neutron reactors is <1%, even after recycling of Pu and RepU. UO2 and MOX fuel technology has matured during the past five decades. These fuels are now being manufactured, used and reprocessed on an industrial scale. Mixed uranium- plutonium monocarbide (MC), mononitride (MN) and U-Pu-Zr alloys are recognized as advanced fuels for sodium cooled fast reactors (SFRs) on the basis of their higher breeding ratio and higher thermal conductivity. The advanced SFR fuels have so far been prepared only on a pilot plant scale in a very few countries, and MA bearing metal, oxide, carbide, nitride and inert matrix fuels are being prepared only on a laboratory scale for property evaluation and irradiation testing. Likewise, thorium based MOX has been manufactured on a pilot plant scale and utilized in power reactors in a few countries in a limited way, but there is no industrial facility for manufacturing these fuels. Until the end of the 1970s, non-power research reactors and their fuels were mostly supplied worldwide by the USA and the former USSR. These reactors used high enriched uranium (HEU) fuel, containing >80% 235U in the form of aluminium matrix, UAlx or U3O8 dispersion fuel of low uranium density (1.3-1.7 g/cm3). In 1978, the USA launched the Reduced Enrichment for Research and Test Reactors (RERTR) Programme, with the objective of converting the HEU core to a low enriched uranium (LEU) core without affecting the operation and performance of the reactors. Later, the Russian Federation also joined this programme. As part of this programme, LEU based Al-U3Si2 dispersion fuel with a uranium density of 4.8 g/cm3 emerged and has been qualified. Efforts are under way to develop advanced fuels such as U-Mo alloy either as Al matrix dispersion fuel with a density of 6-8.5 g/cm3 or as monolithic fuel with a uranium density of 15-16 g/cm3. The IAEA has been fostering information exchange and collaborative R and D among Member States for the development, manufacture and performance evaluation of nuclear fuels for both nuclear power and research reactors, and has published a number of technical reports on nuclear fuels. The purpose of this report is to summarize the current status of nuclear fuel manufacturing technology worldwide for both power reactors and research reactors, and to highlight the trends that are emerging for advanced fuels.
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Aug 2012; 125 p; ISBN 978-92-0-132710-9;
; ISSN 1011-4289;
; Also available on-line: http://www-pub.iaea.org/MTCD/Publications/PDF/TE_1686_web.pdf; Enquiries should be addressed to IAEA, Marketing and Sales Unit, Publishing Section, E-mail: sales.publications@iaea.org; Web site: http://www.iaea.org/books


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Report
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ALUMINIUM, BREEDING RATIO, DISPERSION NUCLEAR FUELS, HIGHLY ENRICHED URANIUM, ISOTOPE PRODUCTION, MEMBER STATES, MIXED OXIDE FUELS, NATURAL URANIUM, PHWR TYPE REACTORS, PILOT PLANTS, PLUTONIUM 239, PLUTONIUM CARBIDES, PLUTONIUM NITRIDES, PLUTONIUM OXIDES, REPROCESSING, RESEARCH REACTORS, SLIGHTLY ENRICHED URANIUM, SODIUM COOLED REACTORS, SPENT FUELS, THERMAL NEUTRONS, THORIUM, THORIUM 232, URANIUM 233, URANIUM 235, URANIUM 238, URANIUM CARBIDES, URANIUM DIOXIDE, URANIUM NITRIDES, URANIUM OXIDES U3O8, URANIUM SILICIDES, URANIUM-MOLYBDENUM FUELS, WATER COOLED REACTORS, WATER MODERATED REACTORS
ACTINIDE COMPOUNDS, ACTINIDE NUCLEI, ACTINIDES, ALLOY NUCLEAR FUELS, ALPHA DECAY RADIOISOTOPES, BARYONS, CARBIDES, CARBON COMPOUNDS, CHALCOGENIDES, CONVERSION RATIO, DIMENSIONLESS NUMBERS, ELEMENTARY PARTICLES, ELEMENTS, ENERGY SOURCES, ENRICHED URANIUM, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FERMIONS, FUELS, FUNCTIONAL MODELS, HADRONS, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, HEAVY WATER COOLED REACTORS, HEAVY WATER MODERATED REACTORS, INTERNAL CONVERSION RADIOISOTOPES, ISOMERIC TRANSITION ISOTOPES, ISOTOPE ENRICHED MATERIALS, ISOTOPES, LIQUID METAL COOLED REACTORS, MATERIALS, METALS, MINUTES LIVING RADIOISOTOPES, NEON 24 DECAY RADIOISOTOPES, NEUTRONS, NITRIDES, NITROGEN COMPOUNDS, NUCLEAR FUELS, NUCLEI, NUCLEONS, OXIDES, OXYGEN COMPOUNDS, PLUTONIUM COMPOUNDS, PLUTONIUM ISOTOPES, PNICTIDES, RADIOISOTOPES, REACTOR MATERIALS, REACTORS, RESEARCH AND TEST REACTORS, SEPARATION PROCESSES, SILICIDES, SILICON COMPOUNDS, SOLID FUELS, SPONTANEOUS FISSION RADIOISOTOPES, THORIUM ISOTOPES, TRANSURANIUM COMPOUNDS, URANIUM, URANIUM COMPOUNDS, URANIUM ISOTOPES, URANIUM OXIDES, YEARS LIVING RADIOISOTOPES
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