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[en] We have demonstrated a generally applicable tabletop approach utilizing a 266nm femtosecond laser pulse pump, 800nm pulse probe, coupled with Coulomb explosion imaging (CEI). We have investigated two simple chemical reactions in C_2H_2"+ simultaneously: proton transfer and C=C bond-breaking, triggered by multiphoton ionization to excited states. Too and fro proton migration results are in excellent agreement with new ab initio trajectory simulations which predict isomerization timescales and pathways. (paper)
Journal
Journal of Physics. Conference Series (Online); ISSN 1742-6596; 
; v. 635(11); [1 p.]
; v. 635(11); [1 p.]