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Aerts, Wouter; De Bruecker, Thomas; Lytek, Anna
American Society of Mechanical Engineers - ASME, Nuclear Engineering Division, Environmental Engineering Division, Two Park Avenue, New York, NY 10016-5990 (United States)2013
American Society of Mechanical Engineers - ASME, Nuclear Engineering Division, Environmental Engineering Division, Two Park Avenue, New York, NY 10016-5990 (United States)2013
AbstractAbstract
[en] Contaminated soils form a large part of the nuclear waste arising from decommissioning activities. The storage and disposal of these large volumes of waste is costly. For this reason techniques which can decontaminate this waste stream to free release levels are economically very interesting. A feasibility study of the possibilities of soil washing to decontaminate such soils was ordered by NIRAS/ONDRAF and performed at Belgoprocess in collaboration with DEC. Initial contamination level and particle size distributions of contaminated soils from three different sources were determined. The main isotopes detected with gamma spectrometry contained in the waste were "2"4"1Am, "1"3"7Cs, "2"2"6Ra, "6"0Co and "2"3"2Th. The particle size distribution revealed that more than half of the mass of the quartz sand that makes up the soil has a particle size between 125 and 212 μm. This fraction is less contaminated than the fractions containing smaller particles. However, separation of the fines fraction (< 125 μm) was not enough to achieve the free release limit. Soil attrition was tested as an extra decontamination step for the sand fraction. The removal efficiencies for the different radionuclides contained in the soil were measured. The process conditions were optimized to achieve maximum removal and a treatment method for the secondary waste coming from this process step was determined. The soil washing process was not only performed with water but also with nitric acid to assess the possibilities of a combination of a mechanical and a chemical decontamination process. Reduction efficiencies of 60-80% for the most relevant radionuclides were recorded. (authors)
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2013; 10 p; ASME; New York, NY (United States); ICEM2013 - ASME 2013: 15. International Conference on Environmental Remediation and Radioactive Waste Management; Brussels (Belgium); 8-12 Sep 2013; ISBN 978-0-7918-5601-7;
; ISBN 978-0-7918-5602-4;
; Available from doi: http://dx.doi.org/10.1115/ICEM2013-96221; Country of input: France; 3 refs


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Book
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Conference
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ACTINIDE NUCLEI, ALKALINE EARTH ISOTOPES, ALPHA DECAY RADIOISOTOPES, AMERICIUM ISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CARBON 14 DECAY RADIOISOTOPES, CESIUM ISOTOPES, CLEANING, COBALT ISOTOPES, EVEN-EVEN NUCLEI, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, HYDROGEN COMPOUNDS, INORGANIC ACIDS, INORGANIC COMPOUNDS, INTERMEDIATE MASS NUCLEI, INTERNAL CONVERSION RADIOISOTOPES, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, MATERIALS, MINERALS, MINUTES LIVING RADIOISOTOPES, NITROGEN COMPOUNDS, NUCLEI, ODD-EVEN NUCLEI, ODD-ODD NUCLEI, OXIDE MINERALS, OXYGEN COMPOUNDS, RADIOACTIVE MATERIALS, RADIOISOTOPES, RADIUM ISOTOPES, SIZE, SPECTROSCOPY, SPONTANEOUS FISSION RADIOISOTOPES, THORIUM ISOTOPES, WASTES, YEARS LIVING RADIOISOTOPES
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