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Chandra, Manish; Ghosh, Suddhasattwa; Venkatesh, P.; Gogoi, Nibedita; Seenivasan, G.; Vandarkuzhali, S.; Nedumaran, S.; Prabhakara Reddy, B.; Nagarajan, K., E-mail: bpreddy@igcar.gov.in
Proceedings of the DAE-BRNS theme meeting commemorating seventy five years of the discovery of Plutonium 2392016
Proceedings of the DAE-BRNS theme meeting commemorating seventy five years of the discovery of Plutonium 2392016
AbstractAbstract
[en] Pyrochemical reprocessing is ideally suited for reprocessing of spent metallic fuels. Molten salt electrorefining is the key step in this process. The separation by electrochemical means is based on the thermodynamic stabilities of the chlorides of actinides and the fission products. The electrochemical behaviour of plutonium in LiCl-KCl eutectic is studied in the present work and compared with the literature data. The electrochemical behavior of Pu"+"3 was studied in the temperature range 748 - 823 K in LiCl-KCl using transient electrochemical techniques, namely, cyclic voltammetry (CV) and chronopotentiometry (CP). The temperature dependence of the diffusion coefficient of Pu"3"+ in LiCl-KCl eutectic and the activation energy were determined in the present work
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Indira Gandhi Centre for Atomic Research, Kalpakkam (India); Board of Research in Nuclear Sciences, Mumbai (India); Indian Association of Nuclear Chemists and Allied Scientists - Southern Regional Chapter, Kalpakkam (India); 230 p; 2016; 2 p; Plutonium 75: DAE-BRNS theme meeting commemorating seventy five years of the discovery of Plutonium 239; Kalpakkam (India); 23-25 May 2016; 4 refs., 3 figs., 1 tab.
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Conference
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