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De Cesare, M.; De Cesare, N.; D’Onofrio, A.; Fifield, L.K.; Gialanella, L.; Terrasi, F., E-mail: m.decesare@cira.it2015
AbstractAbstract
[en] The actinides (e.g. "2"3"6U and "xPu isotopes) are present in environmental samples at the ultra trace level since atmospheric tests of NWs (Nuclear Weapons) performed in the past, deliberate dumping of nuclear waste, nuclear fuel reprocessing, on a large scale and operation of NPPs (Nuclear Power Plants) on a small scale have led to the release of a wide range of radioactive nuclides in the environment. Their detection requires the most sensitive AMS (Accelerator Mass Spectrometry) techniques and at the Center for Isotopic Research on Cultural and Environmental heritage (CIRCE) in Caserta, Italy, an upgraded actinide AMS system, based on a 3-MV pelletron tandem accelerator, has been operated. In this paper the progress made in order to push the "2"3"6U mass sensitivity and "2"3"6U/"2"3"8U isotopic ratio down to the natural levels is reported. A uranium contamination mass of about 0.05 μg and a "2"3"6U/"2"3"8U isotopic ratio sensitivities at the level of 3.2 × 10"−"1"3 are presently achievable.
Primary Subject
Source
AMS-13: 13. accelerator mass spectrometry conference; Aix en Provence (France); 24-29 Aug 2014; S0168-583X(15)00524-8; Available from http://dx.doi.org/10.1016/j.nimb.2015.05.029; Copyright (c) 2015 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Record Type
Journal Article
Literature Type
Conference
Journal
Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms; ISSN 0168-583X;
; CODEN NIMBEU; v. 361; p. 483-487

Country of publication
ACCELERATORS, ACTINIDE NUCLEI, ACTINIDES, ALPHA DECAY RADIOISOTOPES, DETECTION, DIMENSIONLESS NUMBERS, ELECTROSTATIC ACCELERATORS, ELEMENTS, EVEN-EVEN NUCLEI, HEAVY NUCLEI, ISOTOPES, MATERIALS, METALS, NATIONAL ORGANIZATIONS, NUCLEI, RADIOISOTOPES, SPECTROSCOPY, SPONTANEOUS FISSION RADIOISOTOPES, URANIUM ISOTOPES, YEARS LIVING RADIOISOTOPES
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