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Wu, Fengcheng; Lovorn, Timothy; MacDonald, A. H.
Argonne National Laboratory (ANL), Argonne, IL (United States). Funding organisation: USDOE Office of Science - SC, Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division (United States); U.S. Army Research Laboratory - U.S. Army Research Office (ARO) (United States); Welch Foundation (United States); USDOE (United States)2018
Argonne National Laboratory (ANL), Argonne, IL (United States). Funding organisation: USDOE Office of Science - SC, Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division (United States); U.S. Army Research Laboratory - U.S. Army Research Office (ARO) (United States); Welch Foundation (United States); USDOE (United States)2018
AbstractAbstract
[en] In this paper, we present a theory of optical absorption by interlayer excitons in a heterobilayer formed from transition metal dichalcogenides. The theory accounts for the presence of small relative rotations that produce a momentum shift between electron and hole bands located in different layers, and a moire pattern in real space. Because of the momentum shift, the optically active interlayer excitons are located at the moire Brillouin zone's corners, instead of at its center, and would have elliptical optical selection rules if the individual layers were translationally invariant. We show that the exciton moire potential energy restores circular optical selection rules by coupling excitons with different center of mass momenta. A variety of interlayer excitons with both senses of circular optical activity, and energies that are tunable by twist angle, are present at each valley. The lowest energy exciton states are generally localized near the exciton potential energy minima. Finally, we discuss the possibility of using the moire pattern to achieve scalable two-dimensional arrays of nearly identical quantum dots.
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Source
OSTIID--1419946; AC02-06CH11357; Available from https://www.osti.gov/pages/biblio/1419946; DOE Accepted Manuscript full text, or the publishers Best Available Version will be available free of charge after the embargo period
Record Type
Journal Article
Journal
Physical Review B; ISSN 2469-9950;
; v. 97(3); vp

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