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Wang, Rui; Xu, Ya-Qiong; Wang, Tianjiao; Hong, Tu, E-mail: yaqiong.xu@vanderbilt.edu2018
AbstractAbstract
[en] We report a facile method to produce ultrathin molybdenum disulfide (MoS2) hybrids with polarized near-infrared (NIR) photoresponses, in which horizontally-aligned single-walled carbon nanotubes (SWNTs) are integrated with single- and few-layer MoS2 through a two-step chemical vapor deposition process. The photocurrent generation mechanisms in SWNT-MoS2 hybrids are systematically investigated through wavelength- and polarization-dependent scanning photocurrent measurements. When the incident photon energy is above the direct bandgap of MoS2, isotropic photocurrent signals are observed, which can be primarily attributed to the direct bandgap transition in MoS2. In contrast, if the incident photon energy in the NIR region is below the direct bandgap of MoS2, the maximum photocurrent response occurs when the incident light is polarized in the direction along the SWNTs, indicating that photocurrent signals mainly result from the anisotropic absorption of SWNTs. More importantly, these two-dimensional (2D) hybrid structures inherit the electrical transport properties from MoS2, displaying n-type characteristics at a zero gate voltage. These fundamental studies provide a new way to produce ultrathin MoS2 hybrids with inherited electrical properties and polarized NIR photoresponses, opening doors for engineering various 2D hybrid materials for future broadband optoelectronic applications. (paper)
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Source
Available from http://dx.doi.org/10.1088/1361-6528/aaca69; Country of input: International Atomic Energy Agency (IAEA)
Record Type
Journal Article
Journal
Nanotechnology (Print); ISSN 0957-4484;
; v. 29(34); [8 p.]

Country of publication
BOSONS, CARBON, CHALCOGENIDES, CHEMICAL COATING, CRYSTAL LATTICES, CRYSTAL STRUCTURE, CURRENTS, DEPOSITION, ELECTRIC CURRENTS, ELECTROMAGNETIC RADIATION, ELEMENTARY PARTICLES, ELEMENTS, MASSLESS PARTICLES, MATERIALS, MOLYBDENUM COMPOUNDS, NANOSTRUCTURES, NANOTUBES, NONMETALS, PHYSICAL PROPERTIES, RADIATIONS, REFRACTORY METAL COMPOUNDS, SULFIDES, SULFUR COMPOUNDS, SURFACE COATING, TRANSITION ELEMENT COMPOUNDS
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