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AbstractAbstract
[en] Highlights: • Irrigation of a groundwater recharge site with contaminated river water resulted in a three-fold increase of 137Cs-activity in the soil. • 90Sr is more mobile than 137Cs and has reached the gravel layer and presumably permeated into the groundwater. • Irrigation of the recharge field gave an additional input of 30% of 90Sr. • The calculated 239Pu/240Pu atom ratios demonstrate that all plutonium originates from global fallout. • The mass balance for 137Cs shows an additional inventory of 6.000–7.000 Bq/m2 of the recharge soil. This inventory stems from the Chernobyl NPP fallout and from local Swiss NPPs. - Abstract: An important process in the production of drinking water is the recharge of the withdrawn ground water with river water at protected recharge fields. While it is well known that undisturbed soils are efficiently filtering and adsorbing radionuclides, the goal of this study was to investigate their behaviour in an artificial recharge site that may receive rapid and additional input of radionuclides by river water (particularly when draining a catchment including nuclear power plants (NPP)). Soil profiles of recharge sites were drilled and analysed for radionuclides, specifically radiocesium (137Cs), radiostrontium (90Sr) and plutonium (239+240Pu). The distribution of the analysed radionuclides were compared with an uncultivated reference soil outside the recharge site. The main activity of 137Cs was located in the top soil (4.5–7.5 cm) and reached down to a depth of 84 cm and 48 cm for the recharge and the reference site, respectively. The found activities of 239+240Pu originate from the global fallout after 1950. 239+240Pu appeared to be strongly adsorbed onto soil particles. The shape of the depth profile was similar to 137Cs, but also similar between the recharge and the reference site. In contrast, 90Sr showed a uniform distribution over the entire depth of the recharge and reference profiles indicating that 90Sr already entered the gravel zone and the ground water. Elevated inventories of the radionuclides were observed for the recharge site. The soil of the recharge field exhibited a threefold higher activity of 137Cs compared to the reference soil. Also for 239+240Pu higher inventories where observed for the recharge sites (40%). 90Sr behaved differently, showing similar inventories between reference and recharge site. We estimate that 75–89% of the total inventory of 137Cs in the soil at the recharge site (7.000 Bq/m2) originated from the fallout of the Chernobyl accident and from emissions of Swiss NPPs. This estimate is based on the actual activity ratio of 137Cs/239+240Pu of 22 for global fallout. The investigations identified radiostrontium as potential threat to the ground water.
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S0265931X17308238; Available from http://dx.doi.org/10.1016/j.jenvrad.2017.11.019; © 2017 Elsevier Ltd. All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
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Journal Article
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ACTINIDE NUCLEI, ALKALINE EARTH ISOTOPES, ALPHA DECAY RADIOISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CESIUM ISOTOPES, DEVELOPED COUNTRIES, DIMENSIONS, EUROPE, EVALUATION, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FALLOUT, HEAVY NUCLEI, HYDROGEN COMPOUNDS, INTERMEDIATE MASS NUCLEI, ISOTOPES, NUCLEAR FACILITIES, NUCLEI, ODD-EVEN NUCLEI, OXYGEN COMPOUNDS, PLUTONIUM ISOTOPES, POWER PLANTS, RADIOISOTOPES, SPONTANEOUS FISSION RADIOISOTOPES, STRONTIUM ISOTOPES, SURFACE WATERS, THERMAL POWER PLANTS, WATER, WESTERN EUROPE, YEARS LIVING RADIOISOTOPES
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