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Takahashi, Junko; Onda, Yuichi; Hihara, Daichi; Tamura, Kenji, E-mail: takahashi.junko.ka@u.tsukuba.ac.jp2019
AbstractAbstract
[en] Highlights: • 137Cs concentration in soil was fitted by exponential equation at least for 6 y. • Migration from litter to mineral soil was more rapid than in the case of Chernobyl. • 137Cs concentration in surface soil surpassed that of litter within 2–3 y. • Relaxation depth in the two cedar forests has gone down with 0.08 cm y−1. • In contrast, the downward migration in the mixed forest was not clearly observed. - Abstract: After the Fukushima Dai-ichi Nuclear Power Plant accident on March 2011, several studies showed that the downward migration of 137Cs from litter to mineral soil is more rapid in forests in Fukushima than in forests affected by the Chernobyl accident. Therefore, the downward migration within mineral soil layers is more important for predicting long-term dynamics of 137Cs in forest ecosystems in Fukushima. In the present study, we monitored the detailed vertical distribution of 137Cs in litter and soil layers for 6 y (2011–2017) following the previous study (2011–2012), and found that temporal changes in those distributions were different among mixed forest (MF), mature cedar (MC) and young cedar (YC) forests. The 137Cs concentrations and inventories in the litter layer exponentially decreased with time for all sites, with more than 80–95% of the deposited 137Cs on the forest floor distributed in mineral soil layers by 2017. The percentage of 137Cs inventory in the litter layer to the total 137Cs inventory in litter and mineral soil layers was well fitted by a single exponential equation with decreasing rate of 0.22–0.44 y−1. The slower migration was observed in the YC site, probably because of higher initial interception of 137Cs fallout by dense canopy. As the downward migration from litter to mineral soil progressed, the 137Cs concentration in the first few cm of mineral soil surface gradually increased and became higher than the 137Cs concentration in the litter within 2–3 y of the accident. The 137Cs concentration in mineral soil layers exponentially decreased with depth throughout survey period, and an exponential equation fitted well. The relaxation depth of 137Cs concentration in mineral soil layers estimated by the exponential equation were constantly increasing in the MC and YC sites with 0.08 cm y−1. In contrast, there was no temporal increase in the relaxation depth in the MF site, indicating little migration to subsurface soil layer from not only litter layer but also surface soil layer. Further studies are necessary to identify the forests prone to the downward migration of 137Cs and its factors regarding both forest and soil characteristics.
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Source
S0265931X18306490; Available from http://dx.doi.org/10.1016/j.jenvrad.2018.09.009; © 2018 Elsevier Ltd. All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
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Journal Article
Journal
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BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CESIUM ISOTOPES, CONIFERS, DIMENSIONLESS NUMBERS, DIMENSIONS, ECOLOGICAL CONCENTRATION, INTERMEDIATE MASS NUCLEI, ISOTOPES, MEASURING INSTRUMENTS, MONITORS, NUCLEI, ODD-EVEN NUCLEI, PINOPHYTA, PLANTS, RADIOISOTOPES, REACTOR SITES, TREES, YEARS LIVING RADIOISOTOPES
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