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Heine, Daniel; Walther, Clemens; Bister, Stefan, E-mail: heine@irs.uni-hannover.de
18th radiochemical conference. Booklet of abstracts2018
18th radiochemical conference. Booklet of abstracts2018
AbstractAbstract
[en] The vertical distribution of 137Cs, 90Sr, 241Am and plutonium in upper soil layers from the exclusion zone was investigated to get information on the retention mechanisms of these nuclides. Therefore, several drill cores of 30 cm length were collected in the city of Pripyat. Each drill core was cut into 10 layers of different thick-nesses. Due to their half-lives, 137Cs (T1/2=30,17 a) and 90Sr (T1/2=28,78 a) still dominate the contamination in this region. Because of their relevance to long-term considerations the different isotopes of plutonium (238Pu, 239Pu, 240Pu) as well as 241Am being the daughter of 241Pu were also investigated. In the first step, each sample was analyzed by gamma spectrometry to determine the amount of 137Cs and 241Am by their characteristic gamma lines (137Cs: Eγ=661,7 keV; 241Am: Eγ=59,54 keV). In the next steps, the soil samples were ashed and plutonium and strontium were chemically separated. For the detection of plutonium alpha spectrometry was used. The 90Sr measurements were performed by liquid scintillation counting (LSC). The specific activity of 241Am, 137Cs, 90Sr and the three plutonium isotopes in different depths of one drill core are shown in a figure. While the absolute specific activities in layers of equal depth differ considerably, the decrease follows similar slopes in all cores and all nuclide below the 15 cm. Each nuclide is detected down to 30 cm depth. Important information on the different migration behavior is obtained from the specific activity ratios of different nuclides. From the decrease in the ratio of 241Am and 239+240Pu activities migration rates of plutonium and americium are deduced by a simple model.
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Czech Chemical Society, Prague (Czech Republic); 224 p; 2018; p. 181-182; 18. radiochemical conference; Marianske Lazne (Czech Republic); 13-18 May 2018; ISSN 2336-7202;
; Available on-line: https://indico.fjfi.cvut.cz/event/82/attachments/701/913/Booklet_of_Abstracts_CCSSS_162_2018_49_268.pdf; Presented in section 'Radionuclides in the environment, radioecology' as contribution RER.L15 (Id: 707). 2 refs.

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Miscellaneous
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Conference
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ACTINIDE NUCLEI, ALKALINE EARTH ISOTOPES, ALPHA DECAY RADIOISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CAVITIES, CESIUM ISOTOPES, DIMENSIONS, ENRICHED URANIUM REACTORS, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, GRAPHITE MODERATED REACTORS, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, INTERMEDIATE MASS NUCLEI, ISOTOPES, LWGR TYPE REACTORS, NUCLEI, ODD-EVEN NUCLEI, PLUTONIUM ISOTOPES, POWER REACTORS, RADIOISOTOPES, REACTORS, SILICON 32 DECAY RADIOISOTOPES, SPONTANEOUS FISSION RADIOISOTOPES, STRONTIUM ISOTOPES, THERMAL REACTORS, WATER COOLED REACTORS, YEARS LIVING RADIOISOTOPES
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