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Hwang, Inho; Coak, Matthew J; Son, Suhan; Zhang, Kaixuan; Kim, Junghyun; Park, Je-Geun; Lee, Nahyun; Ko, Dong-Su; Oh, Youngtek; Jeon, Insu, E-mail: jgpark10@snu.ac.kr2019
AbstractAbstract
[en] The widely-studied ferromagnetic van-der-Waals (vdW) metal Fe3GeTe2 has great promise for studies of quantum criticality in the 2D limit, but is limited by a relatively high Curie temperature in excess of 200 K. To help render the quantum critical point achievable in such a system within the reach of practically possible tuning methods, we have grown single crystals of a variant of (Fe,Co)3GeTe2 with useful physical properties for both this purpose and the wider study of low-dimensional magnetism and spin transport. (Fe,Co)3GeTe2 is found through x-ray diffraction and electron microscopy to have an equivalent crystal structure to Fe3GeTe2, with a random distribution of the cobalt dopant sites. It exhibits a sharp ferromagnetic transition at a value below 40 K, a stronger anisotropy and a coercive field ten times larger than that of Fe3GeTe2. The transport properties and specific heat show the electronic properties and strong correlations of Fe3GeTe2 to be near-unchanged in this doped material. We demonstrate that (Fe,Co)3GeTe2 can be cleanly exfoliated down to monolayer thickness. This unprecedented hard metallic vdW ferromagnet is a valuable new addition to the limited range of materials available for the study of 2D magnetism. (letter)
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Available from http://dx.doi.org/10.1088/1361-648X/ab3135; Country of input: International Atomic Energy Agency (IAEA)
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Journal Article
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